Nature V_E Microcapsules was produced by using Composite gel method. This method of producing Nature VE Microcapsules was based on the properties of wall material and Complex coacervation process. Gelatin and Alginate were used as wall materials, and 5% of calcium chloride was chose as curing agent. The influence of two different proportion of wall material to Nature V_E Microcapsules Morphology and the effects of particle size distribution and embedding were also researched. The results showed that the production rate and efficiency as well as the solid effective loads were highest when the ratio of gelatin wall at materials: alginate = 31, combining with the shape of produced microencapsulation a rule spherical and particle size distribute appropriate ranging from 30 μm to 60 μm, and the average particle size at 35.17 μm.